For the love of all that is not tacky, stay away from bright colors. Our little two pot calipers aren't worth drawing attention to.
That said, I used a brake caliper paint kit from Autozone on the 2-pots in my old Talon. I went with black and it looked fine years later when I traded it so I could build my Galant. Like any painting job the prep work is everything. I took a wire wheel to mine to clear off any grime and rust and then washed them thoroughly with degreaser before I painted them.
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